According to the dictionary,
2 そのように振る舞う、そのようなふりをする、の意を表す。「偉―・る」「得意―・る」
Expresses that (someone) acts in a certain way or acts a certain way. "To act important." "To act like an expert."
Putting that with the explanation I remember being given by teachers, -tagaru would mean that someone acts in such a way or shows outward signs of wanting to do something. I think most commonly it would be -tagatteiru, because that shows an ongoing state as opposed to a momentary one. You can use it to show that someone has shown that they've wanted to do something for a while now, or was doing it the last time you saw them, whereas -tagaru would be more like they're showing it right at this moment.
Because of those qualities of -tagaru, I think you'd be hard-pressed to use it when someone just said they want to do something, brought it up in passing, or whatever. In those cases -tai to omotteiru or -tai to itteiru would have to be used.
I was going to look this up in whichever Dictionary of Japanese Grammar covers it to be sure, but I just remembered they're a few states away at the moment, so I'm mostly going off of memory here.